Element Selective Probe of the Ultra-Fast Magnetic Response to an Element Selective Excitation in Fe-Ni Compounds Using a Two-Color FEL Source

نویسندگان

  • Eugenio Ferrari
  • Franck Fortuna
  • Franck Vidal
  • Ivaylo Nikolov
  • Paolo Cinquegrana
  • Bruno Diviacco
  • David Gauthier
  • Giuseppe Penco
  • Eléonore Roussel
  • Mauro Trovò
  • Tommaso Pincelli
  • Lounès Lounis
  • Cristian Svetina
  • Marco Zangrando
  • Nicola Mahne
  • Lorenzo Raimondi
  • Michele Manfredda
  • Emanuele Pedersoli
  • Flavio Capotondi
  • Luca Giannessi
  • Maya Kiskinova
  • Giovanni De Ninno
  • Miltcho Boyanov Danailov
  • Enrico Allaria
  • Maurizio Sacchi
چکیده

The potential of the two-color mode implemented at the FERMI free-electron laser (FEL) source for pumping and probing selectively different atomic species has been demonstrated by time-resolved scattering experiments with permalloy (FeNi alloy) and NiFe2O4 samples. We monitored the ultra-fast demagnetization of Ni induced by the pump FEL pulse, by tuning the linearly-polarized FEL probe pulse to the Ni-3p resonance and measuring the scattered intensity in the transverse magneto-optical Kerr effect geometry. The measurements were performed by varying the intensity of the FEL pump pulse, tuning its wavelength to and off of the Fe-3p resonance, and by spanning the FEL probe pulse delays across the 300–900 fs range. The obtained results have Photonics 2017, 4, 6; doi:10.3390/photonics4010006 www.mdpi.com/journal/photonics Photonics 2017, 4, 6 2 of 10 evidenced that for the case of NiFe2O4, there is a sensible difference in the magnetic response at the Ni site when the pump pulse causes electronic excitations at the Fe site.

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تاریخ انتشار 2017